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Jump to main content Jump to site search Publishing * Journals * Books * Databases Search Advanced Search You must enter a search term Advanced search Log in / register ORGANIC CHEMISTRY FRONTIERS View all journals You do not have JavaScript enabled. Please enable JavaScript to access the full features of the site or access our non-JavaScript page. 35 items Top Info Search Recent Articles Published Issues Themed Collections * Previous Issue * View Latest Issue * Next Issue ORGANIC CHEMISTRY FRONTIERS 21 MARCH 2021, ISSUE 6, PAGE 1105 TO 1388 35 items Cover info and contents Cover FRONT COVER -------------------------------------------------------------------------------- Download PDF Cover INSIDE FRONT COVER -------------------------------------------------------------------------------- Download PDF Front/Back Matter CONTENTS LIST -------------------------------------------------------------------------------- Download PDF Research Article SEQUENCE-CONTROLLED SUPRAMOLECULAR COPOLYMER CONSTRUCTED BY SELF-SORTING ASSEMBLY OF MULTIPLE NONCOVALENT INTERACTIONS Hui Li, Ying Yang, Fenfen Xu, Zhaozhao Duan, Riqiang Li, Herui Wen and Wei Tian A sequence-controlled supramolecular copolymer was constructed by self-sorting assembly of metal coordination and two types of host–guest interactions. From the themed collection: FOCUS: Macrocyclic and supramolecular chemistry -------------------------------------------------------------------------------- The article was first published on 28 Jan 2021 Org. Chem. Front., 2021,8, 1117-1124 https://doi.org/10.1039/D0QO01540G Download PDF Article HTML Research Article REMOTE METHYLENE C(SP3)–H FUNCTIONALIZATION ENABLED BY ORGANOPHOSPHINE-CATALYZED ALKYNE ISOMERIZATION De Wang, Zefeng Song, Jianyu Zhang and Tao Xu Non classical EWG-activated arylalkynes as C1 units in organophosphine catalyzed diverse remote sp3 C–H functionalization. -------------------------------------------------------------------------------- The article was first published on 09 Dec 2020 Org. Chem. Front., 2021,8, 1125-1131 https://doi.org/10.1039/D0QO01399D Download PDF Article HTML Research Article HOLE-MEDIATED PHOTOREDOX CATALYSIS: TRIS(P-SUBSTITUTED)BIARYLAMINIUM RADICAL CATIONS AS TUNABLE, PRECOMPLEXING AND POTENT PHOTOOXIDANTS Shangze Wu, Jonas Žurauskas, Michał Domański, Patrick S. Hitzfeld, Valeria Butera, Daniel J. Scott, Julia Rehbein, Ajeet Kumar, Erling Thyrhaug, Jürgen Hauer and Joshua P. Barham Triarylamines are demonstrated as novel, tunable electroactivated photocatalysts that use dispersion precomplexation to harness the full potential of the visible photon (>4.0 V vs. SCE) in anti-Kasha photo(electro)chemical super-oxidations of arenes. From the themed collection: Recent Open Access Articles in Frontiers Journals -------------------------------------------------------------------------------- The article was first published on 03 Mar 2021 Org. Chem. Front., 2021,8, 1132-1142 https://doi.org/10.1039/D0QO01609H Download PDF Article HTML Research Article SYNTHESIS OF POLYCYCLIC NAPHTHOLS AND NAPHTHALENES VIA TANDEM TI(OI-PR)4-PROMOTED PHOTOENOLIZATION DIELS–ALDER REACTION AND AROMATIZATION Xiao-Long Lu, Baochao Yang, Haibing He and Shuanhu Gao An efficient approach to naphthol and naphthalene scaffolds has been developed using a sequence involving tandem Ti(Oi-Pr)4-promoted photoenolization Diels–Alder (PEDA) and aromatization reactions. -------------------------------------------------------------------------------- The article was first published on 04 Jan 2021 Org. Chem. Front., 2021,8, 1143-1148 https://doi.org/10.1039/D0QO01346C Download PDF Article HTML Research Article INTERMOLECULAR ALKENE ARYLCYANATION USING BNSCN AS A CYANIDE SOURCE VIA A REDUCTIVE STRATEGY: ACCESS TO 3,3-DISUBSTITUTED OXINDOLES Yunxia Feng, Shen Zhao, Guopeng Du, Shuang Zhang, Daopeng Zhang, Hui Liu, Xinjin Li, Yunhui Dong and Feng-Gang Sun Herein, a nickel-catalyzed two-component reductive arylcyanation of aryl (pseudo)halide tethered alkenes using benzyl thiocyanate as a cyanide source via C–S bond activation is developed. -------------------------------------------------------------------------------- The article was first published on 06 Jan 2021 Org. Chem. Front., 2021,8, 1149-1154 https://doi.org/10.1039/D0QO01462A Download PDF Article HTML Research Article REGIOSELECTIVE SYNTHESIS OF FUSED OXA-HETEROCYCLES VIA IODINE-MEDIATED ANNULATION OF CYCLIC 1,3-DICARBONYL COMPOUNDS WITH PROPARGYLIC ALCOHOLS Liang Zhang, Neng-Jie Mou, Dong-Rong Xiao, Xin Zhuang, Xiao-Long Lin, Tian Cai and Qun-Li Luo The synthesis of structurally diverse fused oxa-heterocycles is established through the iodine-mediated cascade annulation of cyclic 1,3-dicarbonyl compounds with propargylic alcohols. -------------------------------------------------------------------------------- The article was first published on 11 Jan 2021 Org. Chem. Front., 2021,8, 1155-1162 https://doi.org/10.1039/D0QO01496F Download PDF Article HTML Research Article CONSTRUCTING CHIRAL AZA-QUATERNARY CARBON CENTERS BY ENANTIOSELECTIVE CARBONYLATIVE HECK REACTION OF O-IODOANILINES WITH ALLENES Zhengshuai Xu, Chaoren Shen, Hongru Zhang, Peng Wang and Kaiwu Dong The construction of chiral aza-quaternary C-centers via C–N bond formation is achieved by a Pd-catalysed asymmetric carbonylative Heck reaction of o-iodoanilines with allenes, providing chiral dihydroquinolinone derivatives with moderate to high yield and enantiomeric ratio. -------------------------------------------------------------------------------- The article was first published on 30 Dec 2020 Org. Chem. Front., 2021,8, 1163-1169 https://doi.org/10.1039/D0QO01486A Download PDF Article HTML Research Article FUSED AMBIPOLAR AZA-ISOINDIGOS WITH NIR ABSORPTION Liping Yao, Danlei Zhu, Hailiang Liao, Sheik Haseena, Mahesh Kumar Ravva, Shengyu Cong, Liuyuan Lan, Yazhou Wang, Zhengke Li, Lang Jiang and Wan Yue A series of large and extended novel electron-deficient aza-isoindigos with up to 14 rings was synthesized exhibit excellent solubility, high EA, NIR absorption, planar backbonhole mobility of 0.076 cm2 V−1 s−1 and electron mobility of 0.003 cm2 V−1 s−1. -------------------------------------------------------------------------------- The article was first published on 08 Jan 2021 Org. Chem. Front., 2021,8, 1170-1176 https://doi.org/10.1039/D0QO01495H Download PDF Article HTML Research Article ISOISHWARANE SYNTHASE FROM STREPTOMYCES LINCOLNENSIS Houchao Xu, Jan Rinkel and Jeroen S. Dickschat The product of a terpene synthase from Streptomyces lincolnensis has been identified as the new natural product isoishwarane. The enzyme mechanism was studied by isotopic labelling experiments and site-directed mutagenesis. -------------------------------------------------------------------------------- The article was first published on 19 Jan 2021 Org. Chem. Front., 2021,8, 1177-1184 https://doi.org/10.1039/D0QO01583K Download PDF Article HTML Research Article A NOVEL THREE-COMPONENT REACTION FOR CONSTRUCTING INDOLIZINE-CONTAINING ALIPHATIC SULFONYL FLUORIDES Hong-Ru Chen, Zhen-Yu Hu, Hua-Li Qin and Haolin Tang A copper-catalyzed three-component reaction for transforming quinolines, isoquinolines and pyridines to a class of indolizine-containing alkyl sulfonyl fluorides was developed. -------------------------------------------------------------------------------- The article was first published on 18 Jan 2021 Org. Chem. Front., 2021,8, 1185-1189 https://doi.org/10.1039/D0QO01430C Download PDF Article HTML Research Article RHODIUM(III)-CATALYZED C–H ACTIVATION/ANNULATION OF N-IMINOPYRIDINIUM YLIDES WITH ALKYNES AND DIAZO COMPOUNDS Xiang Li, Ruihong Zhang, Yaoting Qi, Qing Zhao and Tuanli Yao Rh(III)-Catalyzed C–H activation/annulation of N-iminopyridinium ylides with alkynes and diazo compounds has been realized for the synthesis of isoquinolones and isocoumarins. -------------------------------------------------------------------------------- The article was first published on 18 Jan 2021 Org. Chem. Front., 2021,8, 1190-1196 https://doi.org/10.1039/D0QO01333A Download PDF Article HTML Research Article GENERATION OF POWERFUL ORGANIC ELECTRON DONORS BY WATER-ASSISTED DECARBOXYLATION OF BENZIMIDAZOLIUM CARBOXYLATES Guillaume Tintori, Arona Fall, Nadhrata Assani, Yuxi Zhao, David Bergé-Lefranc, Sébastien Redon, Patrice Vanelle and Julie Broggi In situ and easy generation of organic electron donors from water-activation of carboxylate precursors allows OED-promoted intermolecular radical addition reactions. -------------------------------------------------------------------------------- The article was first published on 22 Jan 2021 Org. Chem. Front., 2021,8, 1197-1205 https://doi.org/10.1039/D0QO01488E Download PDF Article HTML Research Article DIAZADIBORININE AS AN AMBIPHILIC CATALYST FOR METAL-FREE HYDROGENATION: A COMPUTATIONAL STUDY ON THE STRUCTURAL DESIGN AND REACTION MECHANISM Youxiang Shao, Ming Huang, Fenglong Gu, Cunyuan Zhao, Ling-Bo Qu and Zhuofeng Ke The reactivity and mechanism of hydrogenation by a metal-free ambiphilic catalyst. -------------------------------------------------------------------------------- The article was first published on 14 Jan 2021 Org. Chem. Front., 2021,8, 1206-1215 https://doi.org/10.1039/D0QO01510E Download PDF Article HTML Research Article A PEGYLATED N-HETEROCYCLIC CARBENE-GOLD(I) COMPLEX: AN EFFICIENT CATALYST FOR CYCLIZATION REACTION IN WATER Bijin Lin, Xumu Zhang, Cong-Ying Zhou and Chi-Ming Che A recyclable, PEGylated N-heterocyclic carbene(NHC)–gold(I) catalyst was synthesized, which exhibited high reactivity and regio-selectivity in the cyclization of alkynoic acids and cascade reaction of tryptamine and alkynoic acids in water. -------------------------------------------------------------------------------- The article was first published on 13 Jan 2021 Org. Chem. Front., 2021,8, 1216-1222 https://doi.org/10.1039/D0QO01266A Download PDF Article HTML Research Article IRIDIUM-CATALYZED ASYMMETRIC HYDROGENATION OF N-PHOSPHINOYLIMINE Congcong Yin, Yingmin Pan, Longsheng Zheng, Bijin Lin, Jialin Wen and Xumu Zhang On catalysis with an iridium tridentate catalyst, prochiral N-phosphinoylimines were hydrogenated with high enantioselectivity and reactivity. An outer-sphere reaction model was proposed in this hydrogenation of CN bonds. -------------------------------------------------------------------------------- The article was first published on 25 Jan 2021 Org. Chem. Front., 2021,8, 1223-1226 https://doi.org/10.1039/D0QO01286F Download PDF Article HTML Research Article VISIBLE LIGHT-MEDIATED CROSS-COUPLING OF ELECTROPHILES: SYNTHESIS OF Α-AMINO AMIDES FROM ISOCYANATES AND KETIMINES Junli Zhu, Cancan Dai, Mengyue Ma, Yanni Yue and Xinyuan Fan Cross-couplings between the electrophilic ketimines and isocyanates are achieved via the visible light-mediated reactivity inversion of the ketimines, affording the desired α-amino amides in high yields, with both metal and metal-free systems. -------------------------------------------------------------------------------- The article was first published on 18 Jan 2021 Org. Chem. Front., 2021,8, 1227-1232 https://doi.org/10.1039/D0QO01620A Download PDF Article HTML Research Article BRØNSTED ACID-CATALYZED HOMOGENEOUS O–H AND S–H INSERTION REACTIONS UNDER METAL- AND LIGAND-FREE CONDITIONS Zhipeng Zhang, Zhiqin He, Yuxing Xie, Tiantong He, Yaofeng Fu, Yang Yu and Fei Huang The economical and accessible CF3SO3H successfully catalyzed homogeneous O–H and S–H bond insertion reactions between hydroxyl compounds, thiols and diazo compounds under metal- and ligand-free conditions. -------------------------------------------------------------------------------- The article was first published on 15 Jan 2021 Org. Chem. Front., 2021,8, 1233-1242 https://doi.org/10.1039/D0QO01401J Download PDF Article HTML Research Article ORGANOCATALYTIC REGIO-, DIASTEREO- AND ENANTIOSELECTIVE Γ-ADDITIONS OF ISOXAZOL-5(4H)-ONES TO Β,Γ-ALKYNYL-Α-IMINO ESTERS FOR THE SYNTHESIS OF AXIALLY CHIRAL TETRASUBSTITUTED Α-AMINO ALLENOATES Fushuai Li, Shuai Liang, Yepeng Luan, Xuling Chen, Hanhui Zhao, Anqi Huang, Pengfei Li and Wenjun Li The chiral phosphoric acid catalyzed regio-, diastereo- and enantioselective reaction of isoxazol-5(4H)-ones with β,γ-alkynyl-α-imino esters has been developed. -------------------------------------------------------------------------------- The article was first published on 20 Jan 2021 Org. Chem. Front., 2021,8, 1243-1248 https://doi.org/10.1039/D0QO01505A Download PDF Article HTML Research Article TRIMERIC AND DIMERIC SESQUITERPENOIDS FROM ARTEMISIA ATROVIRENS AND THEIR CYTOTOXICITIES Li-Hua Su, Tian-Ze Li, Chang-An Geng, Yun-Bao Ma, Xiao-Yan Huang, Jin-Ping Wang, Xue-Mei Zhang and Ji-Jun Chen Two sesquiterpenoid trimers and two sesquiterpenoid dimers possessing unprecedented scaffolds with a methylene-bridged connection were identified from Artemisia atrovirens. Compound 3 showed obvious cytotoxicity against HepG2 and Huh7 cell lines. -------------------------------------------------------------------------------- The article was first published on 22 Jan 2021 Org. Chem. Front., 2021,8, 1249-1256 https://doi.org/10.1039/D0QO01615B Download PDF Article HTML Research Article THEORETICAL STUDY OF RHODIUM- AND COBALT-CATALYZED DECARBOXYLATIVE TRANSFORMATIONS OF ISOXAZOLONES: ORIGIN OF PRODUCT SELECTIVITY Wei Rong, Tian Zhang, Ting Li and Juan Li DFT calculations were performed to elucidate the origins of catalyst-controlled product selectivity in the decarboxylative transformations of isoxazolones. -------------------------------------------------------------------------------- The article was first published on 26 Jan 2021 Org. Chem. Front., 2021,8, 1257-1266 https://doi.org/10.1039/D0QO01498B Download PDF Article HTML Research Article CASCADE INTRAMOLECULAR REARRANGEMENT/CYCLOADDITION OF NITROCYCLOPROPANE CARBOXYLATES WITH ALKYNES/ALKENES: ACCESS TO UNCOMMON BI(HETERO)CYCLIC SYSTEMS Rohit Kumar Varshnaya, Priyanka Singh, Navpreet Kaur and Prabal Banerjee A straightforward approach for the one-pot synthesis of fused bi(hetero)cyclic systems via cascade intramolecular rearrangement/cycloaddition reaction of nitrocyclopropane carboxylates with substituted alkynes/alkenes has been demonstrated. -------------------------------------------------------------------------------- The article was first published on 21 Jan 2021 Org. Chem. Front., 2021,8, 1267-1274 https://doi.org/10.1039/D0QO01535K Download PDF Article HTML Research Article PHTHALIMIDE-BASED-SSCF3 REAGENT FOR ENANTIOSELECTIVE DITHIOTRIFLUOROMETHYLATION Wen-Chao Gao, Jianrong Liu and Xuefeng Jiang A novel dithiotrifluoromethylation reagent phthN-SSCF3 was designed and prepared for the incorporation of a SSCF3 unit into complex molecules and the stereoselective construction of a SSCF3-tethered quaternary carbon center. -------------------------------------------------------------------------------- The article was first published on 22 Jan 2021 Org. Chem. Front., 2021,8, 1275-1279 https://doi.org/10.1039/D1QO00001B Download PDF Article HTML Research Article Α-C–H DIFLUOROALKYLATION OF ALKYL SULFOXIDES VIA INTERMOLECULAR PUMMERER REACTION Xin Huang, Weizhao Zhao, Yuchen Liang, Minghui Wang, Yaling Zhan, Yage Zhang, Lichun Kong, Zhi-Xiang Wang and Bo Peng A simple and practical intermolecular Pummerer reaction using difluoroenol silyl ethers as nucleophiles is described. The protocol allows for highly efficient α-difluoroalkylation of a wide spectrum of alkyl sulfoxides. -------------------------------------------------------------------------------- The article was first published on 22 Jan 2021 Org. Chem. Front., 2021,8, 1280-1287 https://doi.org/10.1039/D0QO01513J Download PDF Article HTML Research Article XANTHANOLTRIMER A–C: THREE XANTHANOLIDE SESQUITERPENE TRIMERS FROM THE FRUITS OF XANTHIUM ITALICUM MORETTI ISOLATED BY HPLC-MS-SPE-NMR Jiang Fu, Ya-Nan Wang, Shuang-Gang Ma, Li Li, Xiao-Jing Wang, Yong Li, Yun-Bao Liu, Jing Qu and Shi-Shan Yu Xanthanoltrimer A–C, first three xanthanolide sesquiterpene trimers from the fruits of Xanthium italicum Moretti, were isolated by HPLC-MS-SPE-NMR. Xanthanoltrimer A–C had an unprecedented 5/7/6/5/7/6/5/7 polycyclic scaffold. -------------------------------------------------------------------------------- The article was first published on 26 Jan 2021 Org. Chem. Front., 2021,8, 1288-1293 https://doi.org/10.1039/D0QO01541E Download PDF Article HTML Highlight MACROCYCLIC AND ACYCLIC SUPRAMOLECULAR ELEMENTS FOR CO-PRECIPITATION OF SQUARE-PLANAR GOLD(III) TETRAHALIDE COMPLEXES Cassandra C. Shaffer and Bradley D. Smith Non-covalent interactions control the solid-state packing of AuX4− anions (yellow circles) co-precipitated with different supramolecular elements. From the themed collection: 2021 Organic Chemistry Frontiers Review-type Articles -------------------------------------------------------------------------------- The article was first published on 28 Jan 2021 Org. Chem. Front., 2021,8, 1294-1301 https://doi.org/10.1039/D0QO01562H Download PDF Article HTML Review Article PHOTOEXCITED MOLECULAR PROBES FOR SELECTIVE AND REVERTIBLE IMAGING OF CELLULAR REACTIVE OXYGEN SPECIES Ying Wen, Zhiqing Long, Fangjun Huo and Caixia Yin Redox homeostasis is key to maintaining the normal physiological status of living cells. From the themed collection: 2021 Organic Chemistry Frontiers Review-type Articles -------------------------------------------------------------------------------- The article was first published on 20 Jan 2021 Org. Chem. Front., 2021,8, 1302-1314 https://doi.org/10.1039/D0QO01260B Download PDF Article HTML Review Article AN ELECTROCHEMICAL PERSPECTIVE ON THE ROLES OF LIGANDS IN THE MERGER OF TRANSITION-METAL CATALYSIS AND ELECTROCHEMISTRY Jun-Song Zhong, Yi Yu, Zhaojiang Shi and Ke-Yin Ye A perspective on the roles of ligands in transition-metal catalysis under electrochemical conditions is provided. From the themed collection: 2021 Organic Chemistry Frontiers Review-type Articles -------------------------------------------------------------------------------- The article was first published on 28 Dec 2020 Org. Chem. Front., 2021,8, 1315-1328 https://doi.org/10.1039/D0QO01227K Download PDF Article HTML Review Article THE OXA-MICHAEL REACTION IN THE SYNTHESIS OF 5- AND 6-MEMBERED OXYGEN-CONTAINING HETEROCYCLES Tauqir Ahmad and Nisar Ullah In this review, we provide an updated account on the recent advances and applications of oxa-Michael reaction in the synthesis 5- and 6-membered monocyclic oxygen-containing heterocyclic compounds published in the literature since 2013 to date. From the themed collection: 2021 Organic Chemistry Frontiers Review-type Articles -------------------------------------------------------------------------------- The article was first published on 19 Jan 2021 Org. Chem. Front., 2021,8, 1329-1344 https://doi.org/10.1039/D0QO01312A Download PDF Article HTML Review Article RECENT ADVANCES IN CASCADE RADICAL CYCLIZATION OF RADICAL ACCEPTORS FOR THE SYNTHESIS OF CARBO- AND HETEROCYCLES Jianhua Liao, Xiao Yang, Lu Ouyang, Yinlong Lai, Jiuzhong Huang and Renshi Luo This review is devoted to highlighting main achievements in the development of cascade radical cyclization of radical acceptors for the synthesis of carbo- and heterocycles. From the themed collection: FOCUS: Radical-involved chemical transformations -------------------------------------------------------------------------------- The article was first published on 08 Jan 2021 Org. Chem. Front., 2021,8, 1345-1363 https://doi.org/10.1039/D0QO01453B Download PDF Article HTML Review Article RECENT ADVANCES IN HYDRIDE TRANSFER-INVOLVED C(SP3)–H ACTIVATION REACTIONS Xiao-De An and Jian Xiao This review summarizes the recent progresses (2016–2020) in the hydride transfer-enabled C(sp3)–H activation according to the reaction types, categorized into the intramolecular/intermolecular C(sp3)–H functionalization, and hydride reduction. From the themed collection: 2021 Organic Chemistry Frontiers Review-type Articles -------------------------------------------------------------------------------- The article was first published on 07 Jan 2021 Org. Chem. Front., 2021,8, 1364-1383 https://doi.org/10.1039/D0QO01502D Download PDF Article HTML Correction CORRECTION: FUSED AMBIPOLAR AZA-ISOINDIGOS WITH NIR ABSORPTION Liping Yao, Danlei Zhu, Hailiang Liao, Sheik Haseena, Mahesh Kumar Ravva, Shengyu Cong, Liuyuan Lan, Yazhou Wang, Zhengke Li, Lang Jiang and Wan Yue From the themed collection: Recent Open Access Articles in Frontiers Journals -------------------------------------------------------------------------------- The article was first published on 03 Mar 2021 Org. Chem. Front., 2021,8, 1384-1385 https://doi.org/10.1039/D1QO90017J Download PDF Article HTML Cover BACK COVER -------------------------------------------------------------------------------- Download PDF 35 items ABOUT ORGANIC CHEMISTRY FRONTIERS High quality research in synthetic methodologies, catalysis, functional organic molecules, organic synthesis and more. 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