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General Review Article
RECENT ADVANCES IN HYDROPHOBIC MODIFICATION OF NANOCELLULOSE
Author(s): Lin Sun, Xiaoyi Zhang, Huayu Liu, Kun Liu, Haishun Du*, Amit Kumar,
Gaurav Sharma* and Chuanling Si*
Volume 25 , Issue 3 , 2021
Published on: 10 December, 2020
Page: [417 - 436] Pages: 20
DOI: 10.2174/1385272824999201210191041
Price: $65
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ABSTRACT
As a kind of renewable nanomaterial, nanocellulose displays excellent
performances and exhibits wide application potentials. In general, nanocellulose
has strong hydrophilicity due to the presence of abundant hydroxyl groups or the
hydrophilic functional groups introduced during the preparation process.
Although these hydrophilic groups benefit the nanocellulose with great
application potential that is used in aqueous media (e.g., rheology modifier,
hydrogels), they do hinder the performance of nanocellulose used as reinforcing
agents for hydrophobic polymers and reduce the stability of the self-assembled
nanostructure (e.g., nanopaper, aerogel) in a high-humidity environment. Thus,
this review aims to summarize recent advances in the hydrophobic modification of
nanocellulose, mainly in three aspects: physical adsorption, surface chemical
modification (e.g., silylation, alkanoylation, esterification), and polymer
graft copolymerization. In addition, the current limitations and future
prospects of hydrophobic modification of nanocellulose are proposed.
Keywords: Nanocellulose, hydrophobic modification, reinforcing agent, cellulose
nanopaper, aerogel, rheology.
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GRAPHICAL ABSTRACT
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CURRENT ORGANIC CHEMISTRY
Title:Recent Advances in Hydrophobic Modification of Nanocellulose
Volume: 25 Issue: 3
Author(s): Lin Sun, Xiaoyi Zhang, Huayu Liu, Kun Liu, Haishun Du*, Amit Kumar,
Gaurav Sharma*Chuanling Si*
Affiliation:
* Tianjin Key Laboratory of Pulp and Paper, Tianjin University of Science and
Technology, Tianjin 300457,China
Keywords: Nanocellulose, hydrophobic modification, reinforcing agent, cellulose
nanopaper, aerogel, rheology.
Abstract: As a kind of renewable nanomaterial, nanocellulose displays excellent
performances and exhibits wide application potentials. In general, nanocellulose
has strong hydrophilicity due to the presence of abundant hydroxyl groups or the
hydrophilic functional groups introduced during the preparation process.
Although these hydrophilic groups benefit the nanocellulose with great
application potential that is used in aqueous media (e.g., rheology modifier,
hydrogels), they do hinder the performance of nanocellulose used as reinforcing
agents for hydrophobic polymers and reduce the stability of the self-assembled
nanostructure (e.g., nanopaper, aerogel) in a high-humidity environment. Thus,
this review aims to summarize recent advances in the hydrophobic modification of
nanocellulose, mainly in three aspects: physical adsorption, surface chemical
modification (e.g., silylation, alkanoylation, esterification), and polymer
graft copolymerization. In addition, the current limitations and future
prospects of hydrophobic modification of nanocellulose are proposed.
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Cite this article as:
Sun Lin , Zhang Xiaoyi , Liu Huayu , Liu Kun , Du Haishun *, Kumar Amit , Sharma
Gaurav *, Si Chuanling *, Recent Advances in Hydrophobic Modification of
Nanocellulose, Current Organic Chemistry 2021; 25(3) .
https://dx.doi.org/10.2174/1385272824999201210191041
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