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* ABSTRACT
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No Access Submitted: 31 October 2020 Accepted: 03 March 2021 Published Online:
25 March 2021
* STRUCTURALLY PHOTO-ACTIVE METAL–ORGANIC FRAMEWORKS: INCORPORATION METHODS,
RESPONSE TUNING, AND POTENTIAL APPLICATIONS
*
Chem. Phys. Rev. 2, 011301 (2021); https://doi.org/10.1063/5.0035739
Nicholas D. Shepherd and Deanna M. D'Alessandroa)
more...View Affiliations
* School of Chemistry, The University of Sydney, Sydney, NSW 2006, Australia
* a)Author to whom all correspondence should be addressed:
deanna.dalessandro@sydney.edu.au
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* Nicholas D. Shepherd
* Deanna M. D'Alessandro
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ABSTRACT
Metal–organic frameworks (MOFs) are an important family of materials due to the
properties that make them well suited to a range of applications. This includes
structurally photo-active MOFs, which have properties that can be efficiently
modulated through controlled light irradiation, making them ideal due to the
cost-effectiveness and noninvasive nature of this stimulus. The incorporation of
structurally photo-active functional groups into MOFs has occurred through
either guest inclusion, as pendant moieties, or as part of a ligand's backbone.
While initial studies into the incorporation of these groups focused on
prominent photo-switches such as azobenzenes, the literature has expanded to
include other classes described in the wider photo-switch literature, most
notably spiropyrans (SPs). The incorporation of alternative photo-switching
classes has currently benefited the field through tuning the light responsive
wavelength. Initial inquiries demonstrated suitable function in gas sorption
applications where irradiation could be exploited for inducing adsorption or
desorption. Furthermore, the potential applications explored in the literature
have also recently expanded to include inquiries into other commercial
functions, such as desalination [R. Ou et al., Nat. Sustain. 3, 1052–1058
(2020)], photo-lithography [H. A. Schwartz et al., Inorg. Chem. 56(21),
13100–13110 (2017)], and drug capture/release [X. Meng et al., Sci. Adv. 2(8),
2–8 (2016)].
ACKNOWLEDGMENTS
We gratefully acknowledge the support of the Australian Research Council (Grant
No. DP180103874). The authors would like to thank the University of Sydney for
resources and facilities necessary for continued research. N.D.S. gratefully
acknowledges the financial support provided by the Postgraduate Scholarship in
Photoactive Metal-Organic Frameworks.
true
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