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Lasing Action with Gold Nanorod Hyperbolic Metamaterials
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Download Hi-Res ImageDownload to MS-PowerPointCite This:ACS Photonics 2017, 4,
3, 674-680
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LASING ACTION WITH GOLD NANOROD HYPERBOLIC METAMATERIALS
* Rohith Chandrasekar†
,
* Zhuoxian Wang†
,
* Xiangeng Meng*†
,
* Shaimaa I. Azzam†
,
* Mikhail Y. Shalaginov†
,
* Alexei Lagutchev†
,
* Young L. Kim‡
,
* Alexander Wei§
,
* Alexander V. Kildishev†
,
* Alexandra Boltasseva†
, and
* Vladimir M. Shalaev*†
View Author Information
† †School of Electrical and Computer Engineering and Birck Nanotechnology
Center, ‡Weldon School of Biomedical Engineering, and §Department of Chemistry,
Purdue University, West Lafayette, Indiana 47907, United States
*E-mail (X. Meng): mengxiangeng@gmail.com
*E-mail (V. M. Shalaev): shalaev@purdue.edu
Cite this: ACS Photonics 2017, 4, 3, 674–680
Publication Date (Web):February 16, 2017
PUBLICATION HISTORY
* Received5 January 2017
* Published online28 February 2017
* Published inissue 15 March 2017
https://doi.org/10.1021/acsphotonics.7b00010
Copyright © 2017 American Chemical Society
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Supporting Info (1)»Supporting Information Supporting Information
SUBJECTS:
* Colloids,
* Lasers,
* Metamaterials,
* Nanorods,
*
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ACS Photonics
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ABSTRACT
Coherent nanoscale photon sources are of paramount importance to achieving
all-optical communication. Several nanolasers smaller than the diffraction limit
have been theoretically proposed and experimentally demonstrated using plasmonic
cavities to confine optical fields. Such compact cavities exhibit a strong
Purcell effect, thereby enhancing spontaneous emission, which feeds into the
lasing modes. However, most plasmonic nanolasers reported so far have employed
relatively narrowband resonant nanostructures and therefore had the lasing
restricted to the proximity of the resonance wavelength. Here, we report on an
approach based on gold nanorod hyperbolic metamaterials for lasing. Hyperbolic
metamaterials provide broadband Purcell enhancement due to the large photonic
density of optical states, while also supporting surface plasmon modes to
deliver optical feedback for lasing due to nonlocal effects in nanorod media. We
experimentally demonstrate the advantage of hyperbolic metamaterials in
achieving lasing action by its comparison with that obtained in a metamaterial
with elliptic dispersion. The conclusions from the experimental results are
supported with numerical simulations comparing the Purcell factors, surface
plasmon modes, and spontaneous emission factors for the metamaterials with
different dispersions. We show that although the metamaterials of both types
support lasing, emission with hyperbolic samples is about twice as strong with
35% lower threshold versus the elliptic ones. Hence, hyperbolic metamaterials
can serve as a convenient platform of choice for nanoscale coherent photon
sources in a broad wavelength range.
KEYWORDS:
* hyperbolic metamaterial
* metal nanorods
* nanolasers
* Purcell enhancement
* nonlocal effect
SUPPORTING INFORMATION
ARTICLE SECTIONS
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* Abstract
* Supporting Information
--------------------------------------------------------------------------------
The Supporting Information is available free of charge on the ACS Publications
website at DOI: 10.1021/acsphotonics.7b00010.
* Fabrication and characterization details, simulated extinction spectra of
nanorod-based metamaterials, isofrequency curves for metamaterials, equations
for calculating the k-space dissipated power density, spectra narrowing and
threshold distribution for nanorod HMM and EMM, emission from glass, gold
film, and lamellar hyperbolic metamaterial samples, local field
distributions, and loss compensation of plasmonic resonance in an HMM (PDF)
* ph7b00010_si_001.pdf (1.4 MB)
Lasing Action with Gold Nanorod Hyperbolic Metamaterials
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