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Hydrogen Peroxide Emission and Fate Indoors during Non-bleach Cleaning: A
Chamber and Modeling Study
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Download Hi-Res ImageDownload to MS-PowerPointCite This:Environ. Sci. Technol.
2020, 54, 24, 15643-15651
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HYDROGEN PEROXIDE EMISSION AND FATE INDOORS DURING NON-BLEACH CLEANING: A
CHAMBER AND MODELING STUDY
* Shan Zhou
Shan Zhou
Department of Chemistry, Syracuse University, Syracuse, New York 13244,
United States
More by Shan Zhou
http://orcid.org/0000-0001-5031-1024
* ,
* Zhenlei Liu
Zhenlei Liu
Department of Mechanical and Aerospace Engineering, Syracuse University,
Syracuse, New York 13244, United States
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* ,
* Zixu Wang
Zixu Wang
Department of Environment and Geography, University of York, York YO10 5DD,
U.K.
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* ,
* Cora J. Young
Cora J. Young
Department of Chemistry, York University, Toronto, Ontario M3J 1P3, Canada
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http://orcid.org/0000-0002-6908-5829
* ,
* Trevor C. VandenBoer
Trevor C. VandenBoer
Department of Chemistry, York University, Toronto, Ontario M3J 1P3, Canada
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http://orcid.org/0000-0001-8926-4237
* ,
* B. Beverly Guo
B. Beverly Guo
Department of Mechanical and Aerospace Engineering, Syracuse University,
Syracuse, New York 13244, United States
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* ,
* Jianshun Zhang
Jianshun Zhang
Department of Mechanical and Aerospace Engineering, Syracuse University,
Syracuse, New York 13244, United States
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* ,
* Nicola Carslaw
Nicola Carslaw
Department of Environment and Geography, University of York, York YO10 5DD,
U.K.
More by Nicola Carslaw
* , and
* Tara F. Kahan*
Tara F. Kahan
Department of Chemistry, Syracuse University, Syracuse, New York 13244,
United States
Department of Chemistry, University of Saskatchewan, Saskatoon, Saskatchewan
S7N 5C9, Canada
*Email: tara.kahan@usask.ca. Tel: (306) 966-1168.
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http://orcid.org/0000-0001-5074-1155
*
Cite this: Environ. Sci. Technol. 2020, 54, 24, 15643–15651
Publication Date (Web):December 1, 2020
PUBLICATION HISTORY
* Received15 July 2020
* Accepted13 November 2020
* Revised4 November 2020
* Published online1 December 2020
* Published inissue 15 December 2020
https://pubs.acs.org/doi/10.1021/acs.est.0c04702
https://doi.org/10.1021/acs.est.0c04702
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SUBJECTS:
* Aldehydes,
* Atmospheric chemistry,
* Kinetic parameters,
* Photodissociation,
* Volatile organic compounds
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ABSTRACT
Activities such as household cleaning can greatly alter the composition of air
in indoor environments. We continuously monitored hydrogen peroxide (H2O2) from
household non-bleach surface cleaning in a chamber designed to simulate a
residential room. Mixing ratios of up to 610 ppbv gaseous H2O2 were observed
following cleaning, orders of magnitude higher than background levels
(sub-ppbv). Gaseous H2O2 levels decreased rapidly and irreversibly, with removal
rate constants (kH2O2) 17–73 times larger than air change rate (ACR). Increasing
the surface-area-to-volume ratio within the room caused peak H2O2 mixing ratios
to decrease and kH2O2 to increase, suggesting that surface uptake dominated H2O2
loss. Volatile organic compound (VOC) levels increased rapidly after cleaning
and then decreased with removal rate constants 1.2–7.2 times larger than ACR,
indicating loss due to surface partitioning and/or chemical reactions. We
predicted photochemical radical production rates and steady-state concentrations
in the simulated room using a detailed chemical model for indoor air (the
INDCM). Model results suggest that, following cleaning, H2O2 photolysis
increased OH concentrations by 10–40% to 9.7 × 105 molec cm–3 and hydroperoxy
radical (HO2) concentrations by 50–70% to 2.3 × 107 molec cm–3 depending on the
cleaning method and lighting conditions.
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SUPPORTING INFORMATION
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* Abstract
* Supporting Information
--------------------------------------------------------------------------------
The Supporting Information is available free of charge at
https://pubs.acs.org/doi/10.1021/acs.est.0c04702.
* Photolysis rate constants of key species in the model; VOC decay rates during
the regular cleaning event; spectral photon flux of two light sources in the
room; modeled and observed H2O2 time series; decay rate constants of H2O2;
H2O2 time series during elevated ventilation periods; NMR results; and
predicted radical concentrations during the deep cleaning event and the
regular cleaning including VOC emissions (PDF)
* es0c04702_si_001.pdf (2.02 MB)
Hydrogen Peroxide Emission and Fate Indoors during Non-bleach Cleaning: A
Chamber and Modeling Study
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